四川大学化学学院
师资力量

徐嘉麒     助理研究员

研究方向:二维固体材料的构筑及其在新能源转化中的应用

联系方式:028-85412904          Email:jqxu@scu.edu.cn

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简历:

学习经历

2010.09–2014.06,天津大学,应用化学,学士,导师:张兵教授

2014.09–2019.06,中国科学技术大学,无机化学,博士,导师:谢毅院士,孙永福教授

工作经历

2019.07–至今,四川大学,无机化学,助理研究员

2019.07–2022.06,四川大学,无机化学,专职博士后,导师:李瑞祥教授

主要研究方向

1. 二氧化碳转化体系研究;

2. 低维固体材料的设计、精准制备以及表征;

3. 催化剂的动态变化过程和反应机理研究;

4. DFT理论计算。

主要工作业绩

随着社会的发展,人类的能源需求和碳排放量都在不断增长。以二氧化碳(CO2)为指标,2019年全球碳排放总量达到了364.41亿吨。CO2的过量排放会造成气候变暖、海水酸化等一系列问题。为了降低社会发展对环境的影响,实现CO2净零排放,我们需要大力发展清洁的碳中和技术。其中,利用半导体催化剂,通过电催化或者光催化的方式将二氧化碳(CO2)和水(H2O)还原得到碳基燃料,是可持续并且环境友好的能源转化与储存方式, 因而具有重要的研究意义。近几年基于电、光催化CO2转化制备碳基燃料及低维固体材料制备等方向上开展了系列研究,目前总共在Nat. EnergyNatl. Sci. Rev.J. Am. Chem. Soc.Angew. Chem. Int. Ed.SCI期刊上发表学术论文16篇,被引超过1800次(H-index 12),申请发明专利6项(授权2项),主持国家自然科学基金青年项目、中国博士后科学基金面上项目等5项科研项目,担任RSC Adv.等期刊的独立审稿人。入选2019年博士后创新人才支持计划,曾获中国科学院院长优秀奖和苏州育才奖等奖励。

主持科研项目

1. 国家自然科学基金委青年科学基金项目:超薄金属性钴基材料的构筑及其红外光催化二氧化碳还原性能研究(2022.01-2024.12, 30)

2. 四川大学专职博士后研发基金项目:超薄铋基材料的构筑及其工业级电流密度下的电催化CO2还原制备液体燃料性能研究(2021.01-2022.12, 12.8)

3. 博士后创新人才支持计划:超薄MXenes材料的电子结构调控及其电催化CO2还原性能的研究(2019.07-2021.06, 60)

4. 中国博士后科学基金面上项目:Cu/MXenes电催化CO2还原材料的设计和制备(2019.12-2021.12, 8)

5. 四川大学博士后交叉学科创新启动基金项目:烟气CO2高效沸石捕集及其电催化制备液体燃料研究(2019.12-2021.12, 10万,共同负责人:王邦达,四川大学建筑与环境学院)

主要奖励和荣誉

2019 中国科学院院长优秀奖

2018 苏州育才奖学金

2016 第二届能源化学与材料国际研讨会:最佳海报奖

2014 新鸿基郭氏励学金

2012 天津大学大学生创新年会优秀项目奖

学术会议

1. 中国化学会第32届学术年会,珠海,2021.04

2. 碳中和技术创新高峰论坛暨四川省碳中和技术创新中心揭牌仪式,成都,2021.04

3. 第四届能源化学与材料国际研讨会,厦门,2018.12

4. 中国化学会第31届学术年会,杭州,2018.05

5. 第二届能源化学与材料国际研讨会,合肥,2016.10

代表性成果 (获奖成果、专著、论文、专利)

1. Jiaqi Xu,+ Xingchen Jiao,+ Kai Zheng,+ Weiwei Shao, Shan Zhu, Xiaodong Li, Junfa Zhu, Yang Pan, Yongfu Sun,* Yi XiePlastics-to-Syngas Photocatalysed by Co-Ga2O3 Nanosheets, Natl. Sci. Rev. 2022, doi.org/10.1093/nsr/nwac011.

2. Shaokun Tao, Shanyong Chen, Meilin Feng, Jiaqi Xu, Maolin Yuan, Haiyan Fu, Ruixiang Li, Hua Chen, Xueli Zheng,* Xiaoqi Yu. Electrochemical Cross-Dehydrogenative Aromatization Protocol for the Synthesis of Aromatic Amines, Org. Lett. 2022, 24, 1011-1016.

3. Jiaqi Xu,* Zhengyu Ju, Wei Zhang, Yang Pan, Junfa Zhu, Jiawei Mao, Xueli Zheng, Haiyan Fu, Maolin Yuan, Hua Chen, Ruixiang Li*. Efficient Infrared‐Light‐Driven CO2 Reduction Over Ultrathin Metallic Ni‐doped CoS2 Nanosheets, Angew. Chem. Int. Ed. 2021, 61, 8705?8709. (Hot Paper)

TOC

4. Li Ji,+ Tianhua Cui,+ Xufeng Nie, Yanling Zheng, Xueli Zheng, Haiyan Fu, Maolin Yuan, Hua Chen, Jiaqi Xu,* Ruixiang Li*. Catalytic Hydrogenation of CO2 with Unsymmetric N-Heterocyclic Carbene-Nitrogen-Phosphine Ruthenium Complexes, Catal. Sci. Technol., 2021, 11, 6965-6969.

5. Wenjing Li, Shun Li, Lihua Luo, Yicen Ge, Jiaqi Xu, Xueli Zheng, Maolin Yuan, Ruixiang Li, Hua Chen and Haiyan Fu*. Visible-Light-Initiated Catalyst-Free Oxidative Cleavage of (Z)-Triaryl-Substituted Alkenes Containing Pyridyl Motif under Ambient Conditions. Green Chem. 2021, 23, 3649–3655.

6. Xingchen Jiao,+ Kai Zheng,+ Qingxia Chen, Xiaodong Li, Yamin Li, Weiwei Shao, Jiaqi Xu, Junfa Zhu, Yang Pan, Yongfu Sun,* Yi Xie*. Photocatalyzing Waste Plastics into C2 Fuels under Simulated Natural Environments. Angew. Chem. Int. Ed. 2020, 59, 15497?15501.

7. Jiaqi Xu,+ Xiaodong Li,+ Zhengyu Ju, Yongfu Sun,* Xingchen Jiao, Ju Wu, Chengming Wang, Wensheng Yan, Huanxin Ju, Junfa Zhu, and Yi Xie*. Visible-Light-Driven Overall Water Splitting Boosted by Tetrahedrally-coordinated Blende CoO Atomic Layers. Angew. Chem. Int. Ed. 2019, 58, 3032-3036.

TOC

8. Xiaodong Li, Yongfu Sun,* Jiaqi Xu, Yanjie Shao, Ju Wu, Xiaoliang Xu, Yang Pan, Huanxin Ju, Junfa Zhu, and Yi Xie*. Selective Visible-Light-Driven Photocatalytic CO2 Reduction to CH4 Mediated by Atomically-thin CuIn5S8 Layers. Nat. Energy 2019, 4, 690-699.

Nat energy 2019

9. Xiaodong Li,+ Liang Liang,+ Yongfu Sun,* Jiaqi Xu, Xingchen Jiao, Xiaoliang Xu, Huanxin Ju, Yang Pan, Junfa Zhu, Yi Xie* . Ultrathin Conductor Enabling Efficient IR Light CO2 Reduction. J. Am. Chem. Soc. 2019, 141, 423-430.

10. Xiaolong Zu,+ Xiaodong Li,+ Wei Liu, Yongfu Sun,* Jiaqi Xu, Tao Yao, Wensheng Yan, Shan Gao, Chengming Wang, Shiqiang Wei, and Yi Xie*. Efficient and Robust Carbon Dioxide Electroreduction Enabled by Atomically Dispersed Snδ+ Sites. Adv. Mater. 2019, 31, 1808135.

11. Ju Wu,+ Xiaodong Li,+ Wen Shi,+ Peiquan Ling, Yongfu Sun,* Xingchen Jiao, Shan Gao, Liang Liang, Jiaqi Xu, Wensheng Yan, Chengming Wang, and Yi Xie* . Efficient Visible-Light-Driven CO2 Reduction Mediated by Defect-Engineered BiOBr Atomic Layers. Angew. Chem. Int. Ed. 2018, 57, 8719?8723.

12. Katong Liu, Xiaodong Li, Liang Liang, Ju Wu, Xingchen Jiao, Jiaqi Xu, Yongfu Sun,* and Yi Xie*. Ni-doped ZnCo2O4 Atomic Layers to Boost the Selectivity in Solar-Driven Reduction of CO2. Nano Res. 2018, 11, 2897?2908.

13. Jiaqi Xu,+ Xiaodong Li,+ Wei Liu,+ Yongfu Sun,* Zhengyu Ju, Tao Yao, Chengming Wang, Huanxin Ju, Junfa Zhu, Shiqiang Wei,* and Yi Xie*. Carbon Dioxide Electroreduction into Syngas Boosted by a Partially Delocalized Charge in Molybdenum Sulfide Selenide Alloy Monolayers. Angew. Chem. Int. Ed. 2017, 56, 9121?9125. (Hot Paper)

Toc

14. Xingchen Jiao,+ Xiaodong Li,+ Xiuyu Jin, Yongfu Sun,* Jiaqi Xu, Liang Liang, Huanxin Ju, Junfa Zhu,Yang Pan, Wensheng Yan, Yue Lin, and Yi Xie*. Partially Oxidized SnS2 Atomic Layers Achieving Efficient Visible-Light-Driven CO2 Reduction. J. Am. Chem. Soc. 2017, 139, 18044?18051.

15. Fengcai Lei,+ Wei Liu,+ Yongfu Sun,* Jiaqi Xu, Katong Liu, Liang Liang, Tao Yao,* Bicai Pan, Shiqiang Wei, Yi Xie*. Metallic Tin Quantum Sheets Confined in Graphene toward High-efficiency CO2 Electroreduction. Nat. Commun. 2016, 7:12697.

16. Fengcai Lei,+ Lei Zhang,+ Yongfu Sun,* Liang Liang, Katong Liu, Jiaqi Xu, Qun Zhang,* Bicai Pan, Yi Luo, and Yi Xie*. Atomic-Layer-Confined Doping for Atomic-Level Insights into Visible-Light Water Splitting. Angew. Chem. Int. Ed. 2015, 54, 9266?9270.

专利

1. 徐嘉麒,李瑞祥,陈华;一种元素掺杂的过渡金属硫化物超薄片及其制备和应用;专利号:ZL 2017 11518682.7

2. 孙永福, 徐嘉麒,谢毅;氧化镓超薄片,其制备方法以及用途;专利号:ZL 201910388370.X

3. 孙永福,徐嘉麒,谢毅;一种氧化亚钴薄片、其制备方法和其在可见光催化全分解水中的应用;专利号:ZL 201810338954 .1

4. 孙永福,徐嘉麒,谢毅;一种过渡金属硫族化合物及其制备方法和应用;专利号:ZL 201710149449.8

5. 熊兰,毛佳伟,徐嘉麒,陈丽先,杨旭东,刘荣,陈思,严峻,郝星杰;一种四核铜配合物及其制备方法和应用;专利号:ZL 202111248730.X

6. 毛佳伟,朱敏,吴宇,徐嘉麒,田华,丁劲松,李铭,王美娜,朱海;一种双核镉配合物及其制备方法和应用;专利号:ZL 202111249975.4

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